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New publication! “Achieving Semi-Metallic Conduction in Al-Rich AlGaN: Evidence of Mott Transition”

June 10, 2024 By Avery-Ryan Ansbro

Abstract: The development of high performance wide-bandgap AlGaN channel transistors with high current densities and reduced Ohmic losses necessitates extremely highly doped, high Al content AlGaN epilayers for regrown source/drain contact regions. In this work, we demonstrate the achievement of semi-metallic conductivity in silicon (Si) doped N-polar Al0.6Ga0.4N grown on C-face 4H-SiC substrates by molecular beam epitaxy. Under optimized conditions, the AlGaN epilayer shows smooth surface morphology and a narrow photoluminescence spectral linewidth, without the presence of any secondary peaks. A favorable growth window is identified wherein the free electron concentration reaches as high as ∼1.8 × 1020 cm−3 as obtained from Hall measurements, with a high mobility of 34 cm2/V·s, leading to a room temperature resistivity of only 1 mΩ·cm. Temperature-dependent Hall measurements show that the electron concentration, mobility, and sheet resistance do not depend on temperature, clearly indicating dopant Mott transition to a semi-metallic state, wherein the activation energy (Ea) falls to 0 meV at this high value of Si doping for the AlGaN films. This achievement of semi-metallic conductivity in Si doped N-polar high Al content AlGaN is instrumental for advancing ultrawide bandgap electronic and optoelectronic devices.

Full text available from Applied Physics Letters

Filed Under: Publications Tagged With: epitaxy, metals, Pat Kezer, transistor

New publication! “Efficient Data Processing Using Tunable Entropy-Stabilized Oxide Memristors“

May 21, 2024 By Avery-Ryan Ansbro

Abstract: Memristive devices are of potential use in a range of computing applications. However, many of these devices are based on amorphous materials, where systematic control of the switching dynamics is challenging. Here we report tunable and stable memristors based on an entropy-stabilized oxide. We use single-crystalline (Mg,Co,Ni,Cu,Zn)O films grown on an epitaxial bottom electrode. By adjusting the magnesium composition (XMg = 0.11–0.27) of the entropy-stabilized oxide films, a range of internal time constants (159–278 ns) for the switching process can be obtained. We use the memristors to create a reservoir computing network that classifies time-series input data and show that the reservoir computing system, which has tunable reservoirs, offers better classification accuracy and energy efficiency than previous reservoir system implementations.

Full text available from Nature Electronics

Filed Under: Publications Tagged With: high entropy, Matt Webb, memristor, Sieun Chae, Tony Chiang

New Publication! “Nernst coefficient of Pt by non-local electrical measurement”

April 9, 2024 By Matt Webb

Abstract: The Nernst effect describes a linear relationship between orthogonal components of a magnetic field, a temperature gradient, and a resulting transverse electric field. A non-local electrical measurement, where injection and detection are physically separated on the specimen, serves as a versatile and effective platform for measuring spin and thermal effects due to the avoided interference with a charge current directly. Here, we quantify the Nernst coefficient of Pt, a common material for spin injection in non-local geometries, by a non-local electrical measurement under modulated temperature and magnetic field and finite element analysis for modeling heat transfer. We determine the Nernst coefficient of Pt from room temperature (8.56 nVK-1 T-1) to 10K (29.3 nVK-1 T-1). Beyond the quantification of the Nernst coefficient, our results show that careful consideration of the thermal properties of the thermal sink and electrode materials is needed when making an interpretation of non-local electrical measurements.

Full text available from Applied Physics Letters

Filed Under: Publications Tagged With: magnetism, Tony Chiang

New Publication! “High temperature stability of entropy-stabilized oxide (MgCoNiCuZn)0.2O in air”

April 9, 2024 By Matt Webb

Abstract: Entropy-stabilized oxides are single-phase, multicomponent oxides that are stabilized by a large entropy of mixing, ΔS, overcoming a positive enthalpy. Due to the −TΔS term in the Gibbs’ free energy, G, it can be hypothesized that entropy-stabilized oxides demonstrate a robust thermal stability. Here, we investigate the high temperature stability (1300–1700 °C) of the prototypical entropy-stabilized rocksalt oxide (MgCoNiCuZn)0.2O in air. We find that at temperatures >1300 °C, the material gradually loses Cu and Zn with increasing temperature. Cu is lost through a selective melting as a Cu-rich liquid phase is formed. Zn is sublimed from the rocksalt phase at approximately similar temperatures to those corresponding to the Cu loss, significantly below both the melting temperature of ZnO and its solubility limit in a rocksalt phase. The elemental loss progressively reduces the entropy of mixing and results in a multiphase solid upon quenching to room temperature. We posit that the high-temperature solubility of Cu and Zn is correlated providing further evidence for entropic stabilization over general solubility arguments.

Full text available from Applied Physics Letters

Filed Under: Publications Tagged With: Avery Ansbro, high entropy, Matt Webb, Peter Meisenheimer, Tony Chiang

New Publication! “Composite Spin Hall Conductivity from Non-collinear Antiferromagnetic Order”

May 4, 2023 By Matt Webb

Abstract: Non-collinear antiferromagnets are an exciting new platform for studying intrinsic spin Hall effects, phenomena that arise from the materials’ band structure, Berry phase curvature, and linear , the spin Hall conductivities in the non-collinear state exhibit the predicted orientation-dependent anisotropy, opening the possibility for new devices with selectable spin polarization. O ur work demonstrates symmetry control through the magnetic lattice as a pathway to tailored functionality in magnetoelectronic systems.

Full text available from Advanced Materials.

Filed Under: Publications Tagged With: magnetism, Nguyen Vu, Pat Kezer, Peter Meisenheimer, Steve Novakov

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News

  • New Publication! “Engineering antiferromagnetic magnon bands through interlayer spin pumping” March 28, 2025
  • New Publication! “Polydopamine-Assisted Electroless Deposition of Magnetic Functional Coatings for 3D-Printed Microrobots” January 31, 2025
  • New Publication! “Geometric effects in the measurement of the remanent ferroelectric polarization at the nanoscale”  January 14, 2025

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About

Our research is at the intersection of multiple disciplines, drawing on principles and methodologies from materials science, chemistry, physics, and electrical engineering. Our mission is to pioneer … Read More

News

New Publication! “Engineering antiferromagnetic magnon bands through interlayer spin pumping”

March 28, 2025 By Avery-Ryan Ansbro

New Publication! “Polydopamine-Assisted Electroless Deposition of Magnetic Functional Coatings for 3D-Printed Microrobots”

January 31, 2025 By Avery-Ryan Ansbro

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